As a group manager, you have total control of each device that has been signed-in to your group. To "add/remove"  devices that belong to your member. Please follow these steps:


1.) In your manager account interface, scroll up a little bit to Group Licenses and click the "Manage License Seats" button.



2.) Then, scroll up a little bit to the member's section and click the "Details" button of the member you want to edit.



Then, you will see the remove button to remove a device. 



Once removed, you can, however, add it back anytime.